IGGCAS OpenIR  > 地球与行星物理院重点实验室
High-Spatial-Resolution Measurement of Water Content in Olivine Using NanoSIMS 50L
Li, Rui-Ying1; Hao, Jialong1; Hu, Sen1; Zhang, Wan-Feng2; Xia, Xiao-Ping2; Lin, Yangting1; Yang, Wei1
2022
Source PublicationATOMIC SPECTROSCOPY
ISSN0195-5373
Volume43Issue:1Pages:77-83
AbstractOlivine is the most abundant mineral in the planetary mantle. Its water content provides critical constraints on the processes and dynamics of the planetary interior. Olivine usually develops zonings with typical widths of 5-20 mu m, which requires high spatial resolution. For secondary ion mass spectrometry (SIMS) measurements, primary beams with low currents were utilized to achieve high spatial resolution. However, this strategy also resulted in high background, which cannot be applied to nominally anhydrous minerals, e.g., olivine. Therefore, achieving high spatial resolution with low background is essential but challenging. For example, even though the NanoSIMS is designed for high-spatial-resolution measurements, the spatial resolution remained at > 10 mu m for water content analysis in order to maintain a low water background of < 10 ppm. In this study, we optimized the primary beam settings and raster size for water content analysis of olivine using a CAMECA NanoSIMS 50L to improve the spatial resolution and the background simultaneously. Olivine standard samples (KLB-1, ICH-30, Mongok) with a water content ranging from 11.2 ppm to 70.6 ppm were measured for water content calibration with H-1-/O-16(-) ratio. San Carlos olivine with a water content of 1.42 ppm was used for background monitoring. The results showed that a spatial resolution of similar to 6 mu m (primary beam size + raster size) with a background of 6 +/- 2 ppm could be achieved by applying a Cs+ beam current of 2 nA with a diameter of similar to 2 mu m, rastering an area of 4 x 4 mu m(2). The analytical reproducibility of this method is better than 13% for standard samples with a water content of > 10 ppm. Overall, this method improved the spatial resolution for measuring water content by a factor of similar to 2 (in comparison to previous studies) and could be applied to olivine grains with complex zoning.
DOI10.46770/AS.2022.005
Funding OrganizationStrategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration
WOS KeywordLUNAR VOLCANIC GLASSES ; HYDROGEN ISOTOPES ; MELT INCLUSIONS ; TRACE-ELEMENTS ; MANTLE ; SIMS ; ZIRCON ; PHOSPHORUS ; VOLATILES ; METEORITE
Language英语
Funding ProjectStrategic Priority Research Program of the Chinese Academy of Sciences[XDB41000000] ; National Key Research and Development Program of China[2018YFA0702601] ; Key Research Program of the Chinese Academy of Sciences[ZDBS-SSW-JSC007-15] ; Key Deployment Program of IGGCAS[IGGCAS202101] ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration[D020203]
Funding OrganizationStrategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; Strategic Priority Research Program of the Chinese Academy of Sciences ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; National Key Research and Development Program of China ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Research Program of the Chinese Academy of Sciences ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Key Deployment Program of IGGCAS ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration ; Pre-research Project on Civil Aerospace Technologies of the China National Space Administration
WOS Research AreaSpectroscopy
WOS SubjectSpectroscopy
WOS IDWOS:000765622700010
PublisherATOMIC SPECTROSCOPY PRESS LTD
Citation statistics
Document Type期刊论文
Identifierhttp://ir.iggcas.ac.cn/handle/132A11/104972
Collection地球与行星物理院重点实验室
Corresponding AuthorHao, Jialong; Yang, Wei
Affiliation1.Chinese Acad Sci, Inst Geol & Geophys, Key Lab Earth & Planetary Phys, Beijing 100029, Peoples R China
2.Chinese Acad Sci, Guangzhou Inst Geochem, State Key Lab Isotope Geochem, Guangzhou 510640, Peoples R China
First Author AffilicationInstitute of Geology and Geophysics, Chinese Academy of Sciences
Corresponding Author AffilicationInstitute of Geology and Geophysics, Chinese Academy of Sciences
Recommended Citation
GB/T 7714
Li, Rui-Ying,Hao, Jialong,Hu, Sen,et al. High-Spatial-Resolution Measurement of Water Content in Olivine Using NanoSIMS 50L[J]. ATOMIC SPECTROSCOPY,2022,43(1):77-83.
APA Li, Rui-Ying.,Hao, Jialong.,Hu, Sen.,Zhang, Wan-Feng.,Xia, Xiao-Ping.,...&Yang, Wei.(2022).High-Spatial-Resolution Measurement of Water Content in Olivine Using NanoSIMS 50L.ATOMIC SPECTROSCOPY,43(1),77-83.
MLA Li, Rui-Ying,et al."High-Spatial-Resolution Measurement of Water Content in Olivine Using NanoSIMS 50L".ATOMIC SPECTROSCOPY 43.1(2022):77-83.
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