IGGCAS OpenIR  > 兰州油气中心
Insights into the effect of humic acid on Ni(II) sorption mechanism on illite: Batch, XPS and EXAFS investigations
Zhao, Xiaolan1,3; Wang, Yun1,3; Wu, Hanyu1; Fang, Linchuan2; Liang, Jianjun1; Fan, Qiaohui1; Li, Ping1
2017-12-01
Source PublicationJOURNAL OF MOLECULAR LIQUIDS
ISSN0167-7322
Volume248Pages:1030-1038
SubtypeArticle
AbstractIn this study, the influence of humic acid (HA) on Ni(II) sorption mechanism at illite/water interface was investigated using batch, EXAFS, and XPS. The results showed that HA can apparently inhibit the sorption of Ni(II) on illite, especially at neutral to weak alkaline conditions under a short aging time. Under low pH conditions, ion exchange (lE) and HA-bridging complexes were the main sorption mechanisms. Under neutral, to weak alkaline conditions, HA-bridging complexes and surface precipitates (such as alpha-Ni(OH)(2)) gradually became predominant for Ni(II) sorption on illite at a short term. The inhibition of HA for Ni(II) sorption was deduced that: (i) the competition of soluble HA-Ni complexes, and (ii) HA-coated illite surface restrained the formation of surface-induced precipitates. With the increasing aging time, the inhibiting effect of HA became weak with respect to the surface precipitates such as Ni-Al LDH and Ni(OH)(2) forming gradually. This might be caused by the growth of the available Al3+ and the surface loading of Ni(II). Moreover, beta-Ni(OH)(2) was the dominant species for Ni(II) sorption on illite under strong alkaline conditions. These findings in this study are providing deep insights into the understanding and prediction of Ni(II) environmental behaviors in soils enriched with natural organic matters. (C) 2017 Elsevier B.V. All rights reserved.
KeywordNi(Ii) Humic Acid Illite Sorption Exafs Xps
WOS HeadingsScience & Technology ; Physical Sciences
DOI10.1016/j.molliq.2017.10.146
Funding OrganizationNatural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009)
WOS KeywordIONIC-STRENGTH ; PRECIPITATE FORMATION ; WATER SUSPENSIONS ; CARBON NANOTUBES ; CLAY-MINERALS ; NI ; MONTMORILLONITE ; ADSORPTION ; NICKEL ; PH
Indexed BySCI
Language英语
Funding OrganizationNatural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009) ; Natural National Science Foundation of China(41573128 ; Natural National Science Foundation of China(41573128 ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Key Laboratory Project of Gansu Province(1309RTSA041) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; Natural Science Foundation of Gansu Province(17JR5RA309) ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; "100-Talent" Program from the Chinese Academy of Sciences in Lanzhou Center for Oil and Gas Resources, Institute of Geology and Geophysics, CAS ; 21601179 ; 21601179 ; 21601169 ; 21601169 ; 21647009) ; 21647009)
WOS Research AreaChemistry ; Physics
WOS SubjectChemistry, Physical ; Physics, Atomic, Molecular & Chemical
WOS IDWOS:000418314400116
PublisherELSEVIER SCIENCE BV
Citation statistics
Cited Times:12[WOS]   [WOS Record]     [Related Records in WOS]
Document Type期刊论文
Identifierhttp://ir.iggcas.ac.cn/handle/132A11/93141
Collection兰州油气中心
Corresponding AuthorFan, Qiaohui; Li, Ping
Affiliation1.Chinese Acad Sci, Inst Geol & Geophys, Gansu Prov Key Lab Petr Resources Res, Key Lab Petr Resources, Lanzhou 730000, Gansu, Peoples R China
2.Northwest A&F Univ, State Key Lab Soil Eros & Dryland Farming Loess P, Yangling 712100, Peoples R China
3.Univ Chinese Acad Sci, Beijing 100049, Peoples R China
Recommended Citation
GB/T 7714
Zhao, Xiaolan,Wang, Yun,Wu, Hanyu,et al. Insights into the effect of humic acid on Ni(II) sorption mechanism on illite: Batch, XPS and EXAFS investigations[J]. JOURNAL OF MOLECULAR LIQUIDS,2017,248:1030-1038.
APA Zhao, Xiaolan.,Wang, Yun.,Wu, Hanyu.,Fang, Linchuan.,Liang, Jianjun.,...&Li, Ping.(2017).Insights into the effect of humic acid on Ni(II) sorption mechanism on illite: Batch, XPS and EXAFS investigations.JOURNAL OF MOLECULAR LIQUIDS,248,1030-1038.
MLA Zhao, Xiaolan,et al."Insights into the effect of humic acid on Ni(II) sorption mechanism on illite: Batch, XPS and EXAFS investigations".JOURNAL OF MOLECULAR LIQUIDS 248(2017):1030-1038.
Files in This Item:
There are no files associated with this item.
Related Services
Recommend this item
Bookmark
Usage statistics
Export to Endnote
Google Scholar
Similar articles in Google Scholar
[Zhao, Xiaolan]'s Articles
[Wang, Yun]'s Articles
[Wu, Hanyu]'s Articles
Baidu academic
Similar articles in Baidu academic
[Zhao, Xiaolan]'s Articles
[Wang, Yun]'s Articles
[Wu, Hanyu]'s Articles
Bing Scholar
Similar articles in Bing Scholar
[Zhao, Xiaolan]'s Articles
[Wang, Yun]'s Articles
[Wu, Hanyu]'s Articles
Terms of Use
No data!
Social Bookmark/Share
Add to CiteULike Add to Connotea Add to Del.icio.us Add to Digg Add to Reddit Add to Technorati
All comments (0)
No comment.
 

Items in the repository are protected by copyright, with all rights reserved, unless otherwise indicated.