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Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA
Fowler, Andrew P. G.1,6; Liu, Qiu-li2,3; Huang, Yongshu2,3; Tan, Chunyang1; Volk, Michael W. R.1,4; Shanks, W. C. Pat, III5; Seyfried, William, Jr.1
2019-11-15
Source PublicationGEOCHIMICA ET COSMOCHIMICA ACTA
ISSN0016-7037
Volume265Pages:148-162
AbstractSulfur isotope values (delta S-34 and Delta S-33) of pyrite in sediment from steam-heated hydrothermal vents on the floor of Yellow-stone Lake ( WY) were measured using secondary ionization mass spectrometry (SIMS). The high resolution of the SIMS data place important constraints on sulfur cycling processes at/near the vent fluid-lake water interface. Pyrite with a distinct mantle-basalt (delta S-34 = 0 parts per thousand) isotope composition (delta S-34 = +0.5 to +3.1 parts per thousand) replaces pyrrhotite during incipient stages of alteration at moderately high temperature. Disseminated cubic pyrite (delta S-34 = +2.0 to +5.3 parts per thousand) occurs in zones where more extensive oxidation is likely. Framboidal pyrite with delta S-34 values ranging from -5.2 to +4.1 parts per thousand and Delta S-33 up to +0.30 parts per thousand suggest formation from low-temperature microbial sulfate reduction in sediments near but not directly in the vent fluid up-flow zone. The co-occurrence of pyrite with S isotope values characteristic of distinct formation processes, coupled with notable intracrystal S isotope variations, suggests the venting locus is dynamic in time and space. (C) 2019 Elsevier Ltd. All rights reserved.
KeywordYellowstone Lake SIMS Sulfur isotopes Pyrite Pyrrhotite Sublacustrine Hydrothermal dynamics
DOI10.1016/j.gca.2019.09.004
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota
WOS KeywordAQUEOUS SULFIDE SOLUTIONS ; SULFATE REDUCTION ; SEDIMENTARY PYRITE ; ISOTOPE FRACTIONATION ; CHIMNEY MINERALS ; HYDROGEN-SULFIDE ; POLYSULFIDE IONS ; S-33 CONSTRAINTS ; STABLE-ISOTOPE ; DEGREES-C
Language英语
Funding ProjectNational Key R&D Program of China[2016YFE0203000] ; NSF[EAR 1515377] ; NSF[OCE 1434798] ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota
Funding OrganizationNational Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota ; National Key R&D Program of China ; National Key R&D Program of China ; NSF ; NSF ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; Instrumentation and Facilities program of the National Science Foundation, Earth Sciences Division ; University of Minnesota ; University of Minnesota
WOS Research AreaGeochemistry & Geophysics
WOS SubjectGeochemistry & Geophysics
WOS IDWOS:000488959900010
PublisherPERGAMON-ELSEVIER SCIENCE LTD
Citation statistics
Document Type期刊论文
Identifierhttp://ir.iggcas.ac.cn/handle/132A11/93928
Collection岩石圈演化国家重点实验室
Corresponding AuthorFowler, Andrew P. G.
Affiliation1.Univ Minnesota, Dept Earth Sci, Minneapolis, MN 55455 USA
2.Chinese Acad Sci, Inst Geol & Geophys, State Key Lab Lithospher Evolut, Beijing 100029, Peoples R China
3.Univ Chinese Acad Sci, Coll Earth Sci, Beijing 100049, Peoples R China
4.Harvard Univ, Dept Earth & Planetary Sci, 20 Oxford St, Cambridge, MA 02138 USA
5.US Geol Survey, Denver Fed Ctr, MS 973, Denver, CO 80225 USA
6.EHS Support, Pittsburgh, PA 15237 USA
Recommended Citation
GB/T 7714
Fowler, Andrew P. G.,Liu, Qiu-li,Huang, Yongshu,et al. Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA[J]. GEOCHIMICA ET COSMOCHIMICA ACTA,2019,265:148-162.
APA Fowler, Andrew P. G..,Liu, Qiu-li.,Huang, Yongshu.,Tan, Chunyang.,Volk, Michael W. R..,...&Seyfried, William, Jr..(2019).Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA.GEOCHIMICA ET COSMOCHIMICA ACTA,265,148-162.
MLA Fowler, Andrew P. G.,et al."Pyrite delta S-34 and Delta S-33 constraints on sulfur cycling at sublacustrine hydrothermal vents in Yellowstone Lake, Wyoming, USA".GEOCHIMICA ET COSMOCHIMICA ACTA 265(2019):148-162.
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